推荐回答(3个)
The result of DME combustion without catalyst is shown in Fig. S1 (Supplementary data, Fig. S1), which indicates that the homogeneous oxidation starts after 200 °C and the temperature for complete conversion is higher than 525 °C. Fig. 1 and Table 1 present the results of the catalytic activities of DME combustion over M-OMS-2 catalysts. It can be seen from Fig. 1 and Table 1 that Co, Ni and Cu doped OMS-2 catalysts exhibit higher catalytic activities compared to Cr and Fe doped OMS-2 catalysts. More importantly, Cu-OMS-2 shows the best activity with the light-off temperature (T10, the temperature acquired for 10% DME conversion) and the full-conversion temperature (T90, the temperature acquired for 90% DME conversion) at 171 and 180 °C, respectively. The temperature window from T10 to T90over Cu-OMS-2 catalyst is less than 10 °C, and this narrow window suggests that Cu-OMS-2 catalyst has excellent low-temperature activity. Considering that the undoped OMS-2 has a T10 of 167°C and a T90 of 213 °C , the T90 for DME combustion has been significantly reduced after doping with transition metals. Over the M-OMS-2 catalysts, CO2 and H2O were the only detectable products within the detection limit.
无催化剂的二甲醚燃烧的结果示于图中。S1(补充数据,图S1),这表明,200℃开始均匀的氧化后,完全转化的温度是高于525℃ 。图1和表1展示M-OMS-2催化剂的催化二甲醚燃烧的结果。从图1和表1中可以看出,Co,Ni和Cu掺杂的OMS-2催化剂表现出更高的催化活性,相比Cr和Fe掺杂的OMS-2催化剂。更重要的是,铜-OMS-2示出了最好的活性在无光温度(T10,获取为10%DME转化率的温度)和完整的转换温度(T90,获得为90%DME转化率的温度),分别在171和180℃。T10至T90以上的Cu-OMS-2催化剂的温度窗口是小于10℃,这个窄的窗口显示的Cu-OMS-2催化剂具有优良的低温活性。认为未掺杂OMS-2的具有一个167℃的T10和213°C的T90,与过渡金属掺杂后的T90为二甲醚燃烧已显着减少。M-OMS-2催化剂,在产品的检出限内CO2和H2O是唯一可检测到的燃烧后物质。
推荐:pdf文件英译汉,可以将内容复制到谷歌翻译,但要注意 换行、特殊符号、文献备注等一些地方需要修改使之成为一个完整正确的句子。翻译出来的汉语也要修改通顺,比自己翻译好多了。
二甲醚燃烧的结果
无催化剂显示
图S1(补充资料,
图S1),这
表明
均相氧化开始
经过200°C和温度
完整的转化率较高
超过525°C.图1和表1
目前的结果
二甲醚燃烧的催化活性
在m-oms-2催化剂。它可以
从图看到。
1、表1
Co,Ni和Cu掺杂的考察
催化剂表现出较高的催化活性—
城市相比,Cr和Fe掺杂
OMS-2催化剂。更重要的—
cu-oms-2不断,显示出最佳的活性与光了
温度(T10,温度
10% DME转化获得—
锡安)和完整的转换
温度(T90,温度
90%二甲醚转化获得的)
在171和180°C,分别。
从T10温度窗口t90over cu-oms-2催化剂
小于10°C,这种狭隘
窗口显示cu-oms-2
催化剂具有优良的
低温活性。考虑到
未掺杂的OMS-2具有T10 167
°C和T90 213°C [ 21 ],
DME燃烧T90
明显fi显著降低后
掺杂过渡金属。
该m-oms-2催化剂,二氧化碳
水是唯一的检测
在检测产品
极限
这是度娘给我的~
图S1(补充数据图S1)显示了无催化剂DEM燃烧的结果,其显示了在200摄氏度以后开始的均相氧化和完成转化时高于525摄氏度的温度。图1和表1显示了DEM在M-OMS-2催化剂下燃烧的催化活性,可以从图1和表1中看出,与Cr和 Fe 混合OMS-2 催化剂相比, Co, Ni 和 Cu混合OMS-2催化剂显示出更高的催化活性。更重要的是,Cu-OMS-2在T10温度(该温度需要10%的DEM转化)和完全转化温度T90(该温度分别需要在117和180摄氏度90%DEM转化)点燃时显示了最好的活性。Cu-OMS-2催化剂在该温度窗口T10到T90小于10摄氏度,该窄窗口示出Cu-OMS-2催化剂具有极好的低温活性。鉴于无掺杂OMS-2在T10处具有167摄氏度在T90具有213摄氏度[21],对于DEM燃烧的T90在掺杂了过渡金属后显著减小。伴随催化剂M-OMS-2,CO2和 H2O是在可检测范围内能检测到的仅有产物。
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